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praseodymium(III) Chloride

PrCl3 salt

Properties

StateSolid (hygroscopic; commonly hydrated)
Colorpale green
SolubilityVery soluble in water; soluble in alcohols
Melting Point803 °C (anhydrous)

About praseodymium(III) Chloride

PrCl3 is the workhorse soluble Pr(III) salt — pale green, hygroscopic, and almost always shipped as the heptahydrate because anyone who has tried to dehydrate it in air knows what happens: instead of clean PrCl3, you get the oxychloride PrOCl and a face full of HCl. The clean route to anhydrous PrCl3 is either vacuum sublimation or the NH4Cl trick — co-melting the hydrate with ammonium chloride under flowing argon, then driving off the ammonium chloride at higher temperature. In the crystal the Pr(III) center sits in a 9-coordinate tricapped trigonal prism, the standard geometry for the larger trivalent lanthanides. The pale green color is diagnostic: weak Laporte-forbidden 4f-4f transitions in the blue (around 450-490 nm) and yellow (570-600 nm) regions of a 4f² ion, with extinction coefficients of only 1-10 M⁻¹ cm⁻¹, leave green light to transmit.

Where you'll encounter it

If you've worked on Pr-doped fiber amplifiers for the 1.3-µm telecom window, the precursor solution that goes into the fluoride-glass fiber preform almost certainly started as PrCl3·7H2O dissolved in dilute HCl. The same salt is the standard feedstock for upconversion phosphors that take infrared excitation and emit visible light — the kind sintered into anti-counterfeiting inks and security taggants. In a synthetic lanthanide-organometallic lab, anhydrous PrCl3 is what you weigh out in the glovebox to make Pr(III) cyclopentadienyl and Pr(III) silylamide complexes. And in any rare-earth pilot plant doing solvent-extraction separations, the chloride is the dissolved form that gets loaded onto the D2EHPA or HEH/EHP organic phase before stripping back into a cleaner aqueous fraction.

Common Uses

  • Precursor for Pr-doped fluoride fiber amplifiers operating in the 1.3-µm telecom window
  • Feedstock for upconversion phosphors used in anti-counterfeiting inks and security taggants
  • Glovebox starting material for Pr cyclopentadienyl and silylamide organometallic complexes
  • Lewis-acid catalyst for Mukaiyama aldol and selected hetero-Diels-Alder reactions
  • Aqueous feed for D2EHPA solvent-extraction separations in rare-earth refining
  • Reduction precursor for Pr metal production via calciothermic or molten-salt electrolysis

Safety Information

GHS classification: Skin irritation Category 2 (H315), Eye irritation Category 2A (H319). Hygroscopic — releases HCl vapor on contact with atmospheric moisture, so weighing in a fume hood with nitrile gloves and splash goggles is standard. No OSHA-specific PEL for praseodymium compounds; the ACGIH lacks a TLV for soluble lanthanide salts but practitioners apply the general particulate-not-otherwise-classified limit of 10 mg/m³ inhalable. Acute oral toxicity is moderate (LD50 in rats around 4500 mg/kg for the trichloride), but the real concern is chronic accumulation in liver and bone if respired as dust over years. Decontaminate spills with damp paper towels rather than dry sweeping to keep dust airborne load down.

This safety summary is for educational reference only and may not be complete. It is not a substitute for Safety Data Sheets (SDS), medical advice, or professional chemical safety guidance. Always consult appropriate SDS and qualified professionals before handling chemicals.

Constituent Elements

Frequently Asked Questions

What is the molar mass of praseodymium(III) chloride?
Anhydrous PrCl3 is 247.258 g/mol (140.908 + 3 × 35.453). The commercial heptahydrate PrCl3·7H2O is 373.366 g/mol — that extra 126 g/mol of water matters when you weigh out a target Pr concentration, so always confirm whether your bottle is the anhydrous or hydrated form before doing the molar arithmetic.
Why is PrCl3 pale green?
Pr(III) has a 4f² ground configuration. Its visible spectrum shows a handful of narrow, weak 4f-4f transitions in the blue (450-490 nm) and yellow (570-600 nm) regions. Because these transitions are Laporte-forbidden, extinction coefficients are tiny — only 1-10 M⁻¹ cm⁻¹ — but they're enough to selectively absorb blue and yellow wavelengths from white light, leaving the complementary green to transmit. The same sharp-line absorption gives lanthanide ions their characteristic pastel colors and razor-thin emission peaks.
Why is anhydrous PrCl3 hard to prepare?
Heating the hydrate in air doesn't drive off water cleanly — it hydrolyzes. Instead of losing H2O, the salt loses HCl and water together, leaving the oxychloride PrOCl as the residue. The clean routes are vacuum sublimation, the NH4Cl method (co-melt the hydrate with excess ammonium chloride under flowing inert gas, then sublime off the NH4Cl), or direct synthesis from Pr metal and Cl2 gas at 500-600 °C. Once you have the anhydrous powder, it has to live in a glovebox or under sealed argon, because it picks up moisture in minutes.