Skip to main content

thulium(III) Chloride

TmCl3 salt

Properties

StateSolid (hygroscopic; commonly hydrated)
Colorpale green
SolubilityVery soluble in water; soluble in alcohols
Melting Point858 °C (anhydrous)

About thulium(III) Chloride

Thulium(III) chloride is a pale-green hygroscopic salt that serves as the standard water-soluble entry point to thulium chemistry — the workhorse precursor for Tm-doped laser crystals, fiber-amplifier dopant solutions, and rare-earth organometallic synthesis. The anhydrous compound adopts the monoclinic AlCl3-type layered structure with each Tm(III) at a 6-coordinate octahedral site of bridging chlorides, although in solution and in the more common heptahydrate TmCl3·7H2O the Tm(III) prefers 8- or 9-coordinate hydration spheres. Anhydrous TmCl3 cannot be made by simply heating the hydrate in air — dehydration always overshoots into thulium oxychloride TmOCl with loss of HCl. The two clean routes are vacuum sublimation around 800°C, or the ammonium chloride method: heat TmCl3·7H2O with a 6-fold excess of NH4Cl under flowing argon, the ammonium chloride sublimes off carrying the water away as NH3·H2O complexes, and the residue is anhydrous TmCl3. The same NH4Cl-assisted dehydration is the standard prep for every lanthanide chloride from LaCl3 to LuCl3. Thulium itself sits at atomic number 69, the second-rarest stable lanthanide (only lutetium is rarer), with crustal abundance around 0.5 ppm — comparable to silver. Tm(III) has a 4f12 configuration, three unpaired electrons, and a sharp electronic emission spectrum dominated by the 1G4 → 3H6 blue line at 475 nm, which is the basis of every Tm-based phosphor and laser system.

Where you'll encounter it

If you've ever had a urologist treat a kidney stone or an enlarged prostate with a thulium fiber laser (TFL) instead of a holmium:YAG laser, the active gain medium in that surgical instrument was thulium-doped silica fiber pumped at 790 nm and lasing at 1940 nm. Tm:YAG and Tm:fiber systems are taking over urology because the 1940-nm wavelength is absorbed by water four times more strongly than holmium's 2120-nm line, giving cleaner ablation with less collateral thermal damage. TmCl3 is the Tm-source feedstock for growing the YAG laser-rod single crystals and for doping the silica preforms that get drawn into fiber. In a research lab, Tm/Yb co-doped upconversion phosphors made from TmCl3 and YbCl3 precursors are the basis of the deep-blue-emitting nanoparticles used as anti-counterfeiting inks and as photodynamic-therapy excitation sources, and the same nanoparticle synthesis is what shows up in security inks on currency printed in the EU and Switzerland.

Common Uses

  • Tm(III) feedstock for growing Tm:YAG and Tm:YLF single-crystal laser rods
  • Doping precursor for Tm-doped silica fiber-amplifier and fiber-laser preforms (1.9-2.1 μm output)
  • Co-precursor (with YbCl3) for synthesis of Tm/Yb upconversion-phosphor nanoparticles
  • Starting material for Tm-Cp* and Tm-amide organometallic complex synthesis
  • Lewis-acid catalyst in research-scale Mukaiyama aldol and Diels-Alder reactions
  • Source for thulium metal production via reduction with calcium or lanthanum at high temperature
  • Calibration standard for ICP-MS analysis of trace thulium in geological samples
  • Doping agent in Tm-based blue phosphors for security inks and anti-counterfeiting tags

Safety Information

GHS: H315 skin irritation (Category 2), H319 eye irritation (Category 2A), H335 respiratory irritation. Acute oral toxicity is moderate (rat LD50 around 480 mg/kg for the chloride). The hydrated salt slowly releases HCl on contact with skin moisture, so prolonged exposure produces mild chemical burns. No OSHA PEL is established specifically for thulium compounds; the rare-earth-element-dust-not-otherwise-specified ACGIH TLV of 10 mg/m3 inhalable dust applies as a default. Chronic inhalation of lanthanide-salt dusts has been linked to a low-grade interstitial pneumonitis in occupational studies of Chinese rare-earth-mining workers. Handle with nitrile gloves, safety glasses, and dust respirator (N95 or better) when weighing the powder; store under desiccation in a tightly closed amber glass bottle to prevent hydration drift.

This safety summary is for educational reference only and may not be complete. It is not a substitute for Safety Data Sheets (SDS), medical advice, or professional chemical safety guidance. Always consult appropriate SDS and qualified professionals before handling chemicals.

Constituent Elements

Frequently Asked Questions

What is the molar mass of thulium(III) chloride?
Anhydrous TmCl3 is 275.29 g/mol: Tm (168.934) + 3 Cl (106.359). The most commonly stocked hydrate is the heptahydrate TmCl3·7H2O at 401.40 g/mol, which is the form supplied by Sigma-Aldrich, Alfa Aesar, and most rare-earth distributors. The hexahydrate at 383.39 g/mol is also documented. When ordering for laser-crystal growth or fiber-doping work, suppliers quote both the elemental Tm content and the hydration state because both affect the dopant stoichiometry.
What is a thulium fiber laser used for in medicine?
Thulium-doped silica fiber lasers emit at 1940 nm, a wavelength absorbed by water about four times more strongly than the 2120-nm holmium:YAG line that dominated urological laser surgery for decades. The stronger water absorption gives a shallower ablation depth (under 200 μm versus 400 μm for Ho:YAG) with less collateral thermal damage, which translates clinically to faster healing and less post-operative pain. Thulium fiber lasers are now standard for benign prostatic hyperplasia (BPH) ablation and for kidney-stone lithotripsy, with companies like Olympus and Quanta System shipping commercial systems. The 1.9-2.0-μm wavelength range also falls in the eye-safe band (above 1.4 μm), which simplifies laser-safety classification.
Why is anhydrous TmCl3 difficult to prepare?
Heating TmCl3·7H2O in air drives off water but the Tm(III)-OH2 hydrolysis equilibrium pushes the system toward thulium oxychloride: TmCl3·7H2O → TmOCl + 6 H2O + 2 HCl. By the time you've heated to 200°C, the residue is contaminated with TmOCl that won't dissolve in dry organic solvents and ruins any subsequent organometallic chemistry. The clean preparation either uses vacuum sublimation of TmCl3 above 800°C to volatilize the chloride away from any oxychloride contaminant, or runs the dehydration in flowing NH4Cl vapor — the NH4Cl decomposes to NH3 and HCl, the HCl suppresses hydrolysis, and the NH3 sweeps water out of the system.